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Observation of a Long-lived Electronic Coherence Modulated by Vibrational Dynamics in Molecular Nd³+- Complexes at Room Temperature

dc.date.accessioned2023-07-24T10:40:23Z
dc.date.available2023-07-24T10:40:23Z
dc.date.issued2023-03-23
dc.identifierdoi:10.17170/kobra-202307248458
dc.identifier.urihttp://hdl.handle.net/123456789/14915
dc.description.sponsorshipGefördert im Rahmen des Projekts DEAL
dc.language.isoeng
dc.rightsAttribution-NonCommercial-NoDerivatives 4.0 International*
dc.rights.urihttp://creativecommons.org/licenses/by-nc-nd/4.0/*
dc.subjectelectronic coherenceeng
dc.subjectfemtochemistryeng
dc.subjectfluorescenceeng
dc.subjectlanthanideseng
dc.subjectwave packetseng
dc.subject.ddc530
dc.subject.ddc540
dc.titleObservation of a Long-lived Electronic Coherence Modulated by Vibrational Dynamics in Molecular Nd³+- Complexes at Room Temperatureeng
dc.typeAufsatz
dcterms.abstractTemporally delayed, phase-locked coherent pairs of near IR femtosecond laser pulses were employed to study electronic coherences in molecular Nd³+-complexes at room temperature. Dissolved and solid complexes were studied under a confocal microscope set-up with fluorescence detection. The observed electronic coherence on a few hundred femtoseconds time scale is modulated by additional coherent wave packet dynamics, which we attribute mainly to be vibrational in nature. In future, the complexes may serve as prototypes for possible applications in quantum information technology.eng
dcterms.accessRightsopen access
dcterms.creatorGhosh, Jayanta
dcterms.creatorGheibi, Mirali
dcterms.creatorKalas, Tillmann
dcterms.creatorSarpe, Cristian
dcterms.creatorZielinski, Bastian
dcterms.creatorCiobotea, Ramela
dcterms.creatorMorscher, Christoph Burghard
dcterms.creatorKoehne, Ingo
dcterms.creatorPietschnig, Rudolf
dcterms.creatorSenftleben, Arne
dcterms.creatorBaumert, Thomas
dcterms.creatorBraun, Hendrike
dcterms.extent7 Seiten
dc.relation.doidoi:10.1002/cphc.202300001
dc.subject.swdKohärenzger
dc.subject.swdFluoreszenzger
dc.subject.swdLanthanoideger
dc.subject.swdWellenpaketger
dc.type.versionpublishedVersion
dcterms.source.identifiereissn:1439-7641
dcterms.source.issueIssue12
dcterms.source.journalChemPhysChemeng
dcterms.source.volumeVolume 24
kup.iskupfalse
dcterms.source.articlenumbere202300001


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