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Please use this identifier to cite or link to this item: http://nbn-resolving.de/urn:nbn:de:hebis:34-2008102924934

Title: Femtosecond two-photon ionization spectroscopy of the B state of Na_3 clusters
Authors: Baumert, ThomasThalweiser, RainerGerber, Gustav
???metadata.dc.subject.ddc???: 530 - Physik (Physics)
Issue Date: 1993
Citation: In: Chemical physics letters. - Amsterdam : North-Holland Publ. Co., 209.1993, S. 29-34
Abstract: We report time-resolved experiments studying the dynamics of the Na_3 B-X system. Femtosecond pump-probe techniques combined with ion time-of-flight (TOF) and zero kinetic energy (ZEKE) photoelectron spectroscopy allow us to observe the three-dimensional wavepacket motion in the excited Na_3 B state and in the Na_3 X state. The ground state wavepacket is induced by stimulated emission pumping during the pump pulse. The X-state dynamics is dominated by the three vibrational modes of the Na_3. Furthermore we observed pseudorotational wavepacket motion in the B state. We do not observe a fragmentation of the B state within a time interval of 10 ps.
URI: urn:nbn:de:hebis:34-2008102924934
ISSN: 0009-2614
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